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作者 : Yi-Yun Yu ;   Gunda I. Georg ;  
ISSN : 1615-4150;1615-4169;
出版时间 : 2014
卷期 : 356(6)
起始页码 : 1359
终止页码 : 1369
摘要 : A green and mild protocol for the dehydrogenative olefination of cyclic enaminones was devised via palladium catalysis at room temperature using oxygen as the terminal oxidant. The synthetic utility of the olefinated cyclic enaminones afforded a series of unique 1,3,5-trisubstituted benzenes via an unanticipated Diels-Alder tandem reaction. The broad substrate scope and good yields achieved with this new protocol provide an alternative pathway for arene functionalization.


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N-Heterocyclic Carbene-Catalyzed Reaction of Alkynyl Aldehydes with 1,3-Keto Esters or 1,3-Diketones期刊论文

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Titanium-Mediated Direct Carbon-Carbon Double Bond Formation to alpha-Trifluoromethyl Acids: A New Contribution to the Knoevenagel Reaction and a High-Yielding and Stereoselective Synthesis of alpha-Trifluoromethylacrylic Acids期刊论文

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Highly Efficient Asymmetric Epoxidation of Electron-Deficient alpha,beta-Enones and Related Applications to Organic Synthesis期刊论文

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Highly Enantioselective Epoxidation of alpha,beta-Unsaturated Ketones Catalyzed by Primary-Secondary Diamines期刊论文

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Facile, Efficient Copolymerization of Ethylene with Bicyclic, Non-Conjugated Dienes by Titanium Complexes Bearing Bis(beta-Enaminoketonato) Ligands期刊论文

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N,N,N ',N '-Tetramethylchloroformamidinium Chloride-Mediated Cyclizations of beta-Oxo Amides: Facile and Divergent One-Pot Synthesis of Substituted 2H-Pyrans, 4H-Pyrans and Pyridin-2(1H)-ones期刊论文

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Impact of carbon dioxide pressurization on liquid phase organic reactions: A case study on Heck and Diels-Alder reactions期刊论文

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Impact of Carbon Dioxide Pressurization on Liquid PhaseOrganic Reactions: A Case Study on Heck and Diels–AlderReactions期刊论文

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