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作者 : Yi-Yun Yu ;   Gunda I. Georg ;  
ISSN : 1615-4150;1615-4169;
出版时间 : 2014
卷期 : 356(6)
起始页码 : 1359
终止页码 : 1369
摘要 : A green and mild protocol for the dehydrogenative olefination of cyclic enaminones was devised via palladium catalysis at room temperature using oxygen as the terminal oxidant. The synthetic utility of the olefinated cyclic enaminones afforded a series of unique 1,3,5-trisubstituted benzenes via an unanticipated Diels-Alder tandem reaction. The broad substrate scope and good yields achieved with this new protocol provide an alternative pathway for arene functionalization.

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